the letter today itself, it's urgent.
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I've never heard today itself and without your explanation, I would have no idea what it means. So I would recommend avoiding it. It seems to me that "You have to do this work today" or "You have to get this work done today" are quite clear without any further modification, but if you really wanted to emphasize "today," there is more than one way to do so, e.g., "You must complete this by the end of today at the latest" or "by the end of the day at the latest."
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