The swimming pool of the Great Bath was made watertight with burnt bricks and mortar lined with bitumen and
a)lime
b)gypsum
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I think gypsum is the answer
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The floor of the tank was watertight due to finely fitted bricks laid on edge with a gypsum plaster, and the side walls were constructed in a similar manner. To make the tank even more watertight, a thick layer of bitumen (waterproof tar) was laid along the sides of the pool and presumably also on the floor.
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