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The formation of Li3N can be explained thermodynamically. The enthalpy of formation of the N3− ion is extremely endothermic (it involves three successive additions of electrons) and with the larger counterions Na+ or K+ the lattice energy (which is proportional to q+q−r++r−) is not sufficiently large to compensate for the large ΔfH of N3−. The same argument explains why magnesium also forms a nitride.
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